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Nanopore creation in graphene at the nanoscale for water desalination.

Article scientifique 2023 Anglais

Résumé

Abstract Creating nanopores in graphene is a powerful tool for engineering its properties. Nanopores in graphene tune their electrical, optical, magnetic, and mechanical properties. However, controlling nanopores formation at the nanoscale level remains a significant challenge. We report an easy method to control nanopore sizes using argon-plasma magnetron sputtering. By calculating and measuring Raman spectra, we show that the nano-pores in graphene are controllable and size-tunable. Furthermore, we report that the graphene Raman mode around 1450 cm-1 is only due to nanopores and was attributed to the substrate effect. Here, we also propose a novel graphene device-based water filtration. Our proposed concept of two graphene electrodes with nanopores on the substrate (SiC and SiO2) makes it possible to have the highest permeability value, keeping a 100 % salt rejection and improving its mechanical properties. These reported results are essential for developing water desalination membranes based on graphene devices.

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Abdelkader, S., Benabdallah, I., Amlieh, M., Fatimy, A. (2023). Nanopore creation in graphene at the nanoscale for water desalination.. https://doi.org/10.21203/rs.3.rs-2982389/v1

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