Design and implementation of PLA/GO/metal oxide composites for CO2 sensing application

Résumé

This study investigates the modification of polylactic acid (PLA) by the incorporation of graphene oxide (GO) and metal oxides (ZnO and CuO), with the aim of developing efficient CO₂ sensors. Key properties, including total dipole moment (TDM), energy gap (ΔE), molecular electrostatic potential (MESP), and density of states (DOS), were calculated using density functional theory (DFT) to gain insight into the interactions between the composites and CO₂ gas. Experimental techniques such as X-ray diffraction (XRD), Fourier transform infrared spectroscopy (FTIR), and optical confocal microscopy were used to validate the material composition and bonding mechanisms. The analysis revealed the presence of SiO₂ impurities in the PLA matrix, which could potentially affect the sensing behavior of the composite. The composites demonstrated effective CO₂ sensing capabilities in experimental tests. This combined theoretical and experimental approach demonstrates that PLA/GO/metal oxide composites offer significant potential for sustainable CO₂ sensing, contributing to air quality monitoring and greenhouse gas regulation.

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